I found this article that states the problem of the alternator pulley...
"On the early days of their serpentine belt implementation on the AAZ engine (MK3 chassis 1993+) VW used a standard (solid) alternator pulley, meaning that the alternator is directly connected to the crankshaft drive pulley via a serpentine belt.
This engine (and its gasser cousins the ABA and VR6) unfortunately became a bit infamous for wearing out the crankshaft sprocket, key, and keyway. It’s generally accepted that a large contributing factor to this problem was that the alternator has a small pulley and a lot of angular momentum; during deceleration it tends to want to overdrive the engine, putting large stresses on the crankshaft drive pulley (and the keyway) therein in a direction opposite to normal. Over time acceleration and deceleration results in the crankshaft sprocket rocking loose… on a diesel the result can be catastrophic. The small pulley on the alternator exacerbates the problem (over previous designs) by increasing the alternator RPM and giving it a mechanical advantage when overdriving the larger crankshaft pulley.
At some point just before they moved to the TDI engine VW switched to a 1-way ratcheting alternator pulley (which they continued with on the TDI engine). This pulley allows the alternator to automatically de-clutch from the drivebelt and freewheel on its own… preventing the alternator from applying reverse torque to the crankshaft pulley when the engine decelerates."
Another place they speak of a solid pulley ruining the vibration damper. Which would or could break the crankshaft. I have seen this first hand on the larger diesel engines.
But, any rotating mass changes do affect things in different ways. Vibrations at the right frequencies do strange things.
And, don't take me wrong, I do like to modify stuff if it does good or helps. If you want to try it out I would love to hear about the results both short term and long term. I love driving my single mass flywheel cars and they have done me well for many miles.