You need to use VCDS/Vag-Com/or something equivalent to look at the different measuring blocks in the ECU and read any relevant codes.- so that's great you wired up the ODB plug.
I would start by checking out what it is seeing for TPS input - to confirm if it's understanding your request for more throttle. The wiring for the pedal swap can tricky, there is some conflicting information out there on it.
If it starts and runs you have the essentials connected. Issues with the N75, lack of MAF, EGR, etc will not keep you from (slowly albeit) going through the rev range. Some brake switch faults, and issues with the TPS will cause that behavior. A bad injection pump QA, or possibly too high of an injection pump IQ might also.
How's it run between idle and 1500-2000 rpm? Is it a hard cut or does it start to stumble/bog?